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Josephson scanning tunneling microscopy (JSTM) is a powerful probe of the local superconducting order parameter, but studies have been largely limited to cases where the superconducting sample and superconducting tip both have the same gap symmetry—either s-wave or d-wave. It has been generally assumed that, in an ideal s-to-d JSTM experiment, the critical current would vanish everywhere, as expected for ideal c-axis planar junctions. We show here that this is not the case. Employing first-principlesWannier functions for Bi2Sr2CaCu2O8+δ , we develop a scheme to compute the Josephson critical current (Ic) and quasiparticle tunneling current measured by JSTM with subangstrom resolution. We demonstrate that the critical current for tunneling between an s-wave tip and a superconducting cuprate sample has the largest magnitude above O sites and it vanishes above Cu sites. Ic changes sign under π/2 rotation and its average over a unit cell vanishes, as a direct consequence of the d-wave gap symmetry in cuprates. Further, we show that Ic is strongly suppressed in the close vicinity of a Zn-like impurity owing to suppression of the superconducting order parameter. More interestingly, Ic acquires nonvanishing values above the Cu sites near the impurity. The critical current modulations produced by the impurity occur at characteristic wave vectors distinct from the quasiparticle interference (QPI) analog. Furthermore, the quasiparticle tunneling spectra in the JSTM setup shows coherence peaks and impurity-induced resonances shifted by the s-wave tip gap. We discuss the similarities and differences in JSTM observables and conventional STM observables, making specific predictions that can be tested in future JSTM experiments. 

Abstract An unidentified quantum fluid designated the pseudogap (PG) phase is produced by electron-density depletion in the CuO 2 antiferromagnetic insulator. Current theories suggest that the PG phase may be a pair density wave (PDW) state characterized by a spatially modulating density of electron pairs. Such a state should exhibit a periodically modulating energy gap $${\Delta }_{{{{{{\rm{P}}}}}}}({{{{{\boldsymbol{r}}}}}})$$ Δ P ( r ) in real-space, and a characteristic quasiparticle scattering interference (QPI) signature $${\Lambda }_{{{{{{\rm{P}}}}}}}({{{{{\boldsymbol{q}}}}}})$$ Λ P ( q ) in wavevector space. By studying strongly underdoped Bi 2 Sr 2 CaDyCu 2 O 8 at hole-density ~0.08 in the superconductive phase, we detect the 8 a 0 -periodic $${\Delta }_{{{{{{\rm{P}}}}}}}({{{{{\boldsymbol{r}}}}}})$$ Δ P ( r ) modulations signifying a PDW coexisting with superconductivity. Then, by visualizing the temperature dependence of this electronic structure from the superconducting into the pseudogap phase, we find the evolution of the scattering interference signature $$\Lambda ({{{{{\boldsymbol{q}}}}}})$$ Λ ( q ) that is predicted specifically for the temperature dependence of an 8 a 0 -periodic PDW. These observations are consistent with theory for the transition from a PDW state coexisting with d -wave superconductivity to a pure PDW state in the Bi 2 Sr 2 CaDyCu 2 O 8 pseudogap phase. 

The defining characteristic of hole-doped cuprates is d -wave high temperature superconductivity. However, intense theoretical interest is now focused on whether a pair density wave state (PDW) could coexist with cuprate superconductivity [D. F. Agterberg et al., Annu. Rev. Condens. Matter Phys. 11, 231 (2020)]. Here, we use a strong-coupling mean-field theory of cuprates, to model the atomic-scale electronic structure of an eight-unit-cell periodic, d -symmetry form factor, pair density wave (PDW) state coexisting with d -wave superconductivity (DSC). From this PDW + DSC model, the atomically resolved density of Bogoliubov quasiparticle states N r , E is predicted at the terminal BiO surface of Bi 2 Sr 2 CaCu 2 O 8 and compared with high-precision electronic visualization experiments using spectroscopic imaging scanning tunneling microscopy (STM). The PDW + DSC model predictions include the intraunit-cell structure and periodic modulations of N r , E , the modulations of the coherence peak energy Δ p r , and the characteristics of Bogoliubov quasiparticle interference in scattering-wavevector space q - space . Consistency between all these predictions and the corresponding experiments indicates that lightly hole-doped Bi 2 Sr 2 CaCu 2 O 8 does contain a PDW + DSC state. Moreover, in the model the PDW + DSC state becomes unstable to a pure DSC state at a critical hole density p *, with empirically equivalent phenomena occurring in the experiments. All these results are consistent with a picture in which the cuprate translational symmetry-breaking state is a PDW, the observed charge modulations are its consequence, the antinodal pseudogap is that of the PDW state, and the cuprate critical point at p * ≈ 19% occurs due to disappearance of this PDW.